Leo Compatibility with All 12 Zodiac Signs Best to WorstLibra passion most suitable zodiac signs are twins, water bearer, and aries. When it comes to matters of the love, Libra seeks harmony and compatibility above all else. Gemini can offer stimulation and fun to the connection, while The Water Bearer shares Libra's appreciation for wisdom and originality. The Ram, known for their intensity, can ignite a spark in Libra's spirit. Libra and these signs create a balanced and fulfilling partnership.